دوره 12، شماره 2 - ( 12-1403 )
جلد 12 شماره 2 صفحات 151-137 |
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Shirvani F, Morad-Alizadeh S, Rezaei M. Investigation of Advanced Oxidation Processes Based on Ultraviolet Radiation for the Removal of Phthalate Compounds from Aquatic Environments. J Environ Health Eng 2025; 12 (2) :137-151
URL: http://jehe.abzums.ac.ir/article-1-1077-fa.html
URL: http://jehe.abzums.ac.ir/article-1-1077-fa.html
شیروانی فاطمه، مرادعلی‌زاده سعیده، رضایی مهدی. بررسی روشهای اکسیداسیون پیشرفته بر پایه اشعه فرابنفش جهت حذف ترکیبات فتالات از محیط های آبی. مجله مهندسی بهداشت محیط. 1403; 12 (2) :137-151
مرکز تحقیقات مهندسی بهداشت محیط، دانشگاه علوم پزشکی کرمان، کرمان، ایران & گروه مهندسی بهداشت محیط، دانشکده بهداشت، دانشگاه علوم پزشکی کرمان، کرمان، ایران
چکیده: (215 مشاهده)
زمینه و هدف: فتالات‌ها از جمله مهم‌ترین آلاینده‌های صنعتی بوده که سلامت انسان را به خطر می‌اندازند. این ترکیبات مختل‌کننده غدد درون‌ریز، معمولاً در ساخت اثاثیه و ظروف پلاستیکی کاربرد دارند که از طریق جریان فاضلاب، به راحتی وارد منابع آب می‌شوند. از میان روشهای حذف این نوع آلاینده از محیط‌های آبی، روشهای اکسیداسیون پیشرفته فتوشیمیایی، توجه زیادی را به خود جلب کرده‌است؛ لذا هدف از انجام مطالعه حاضر، بررسی و مقایسه روشهای اکسیداسیون پیشرفته بر پایه اشعه فرابنفش جهت حذف ترکیبات فتالات از محیط‌های آبی بود.
مواد و روش ها: برای انجام مطالعه مروری حاضر، پس از جست‌وجوی کلیدواژه‌ها در پایگاه‌های داده «ScienceDirect, SID, Magiran, PubMed, Wiley, Springer»، از ژانویه سال ۲۰۱۳ تا دسامبر ۲۰۲۴ میلادی، جمعاً ۶۹۳ مقاله یافت شد که پس از انجام مراحل غربالگری و بررسی کامل مقالات، در نهایت تعداد ۵۴ مقاله ثبت و در مطالعه استفاده شد. معیار ورود مقالات به مطالعه؛ شامل بررسی نحوه ورود ترکیبات فتالات به محیط زیست، اثرات بهداشتی و نیز تشریح فرایندهای اکسیداسیون پیشرفته در کنار بررسی مزایا و معایب این فرایندها بود.
یافته ها: تابش اشعه فرابنفش می‌تواند به تنهایی ترکیبات فتالات را تا حدودی از بین ببرد. با این حال، این تابش در برابر حذف بسیاری از این ترکیبات بی‌اثر است؛ بنابراین، حذف مؤثر ترکیبات فتالات با این روش، مستلزم ترکیب تابش اشعه ماوراء بنفش با اکسیدان‌ها است. روشهای مختلفی از فرایند اکسیداسیون پیشرفته بر پایه اشعه فرابنفش وجود دارد که عمدتاً شاملUV/H2O2 ,UV/H2O2/Fe+3, UV/Cl-, UV/persulfate, UV/H2O2/Fe+2 UV/Cl-cyanurates ,oxalate, UV/TiO2, UV/Cl-/TiO2, UV/O3 می‌شوند؛ اما به طور کلی، می‌توان گفت که فرایند «فرابنفش/کلر-سیانورات» به عنوان اقتصادی‌ترین فرایند اکسیداسیون پیشرفته بر پایه اشعه فرابنفش شناخته می‌شود.
نتیجه گیری: پس از بررسی خصوصیات و عملکرد فرایندهای مذکور برای حذف ترکیبات فتالات از محیط‌های آبی، در نهایت فرایند «فرابنفش/کلر-سیانورات» به دلیل مصرف انرژی کمتر، مقرون‌به‌صرفه اقتصادی بودن و خصوصاً راندمان حدف تقریباً ۱۰۰ درصد پیشنهاد گردید.
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